Direct decarbonization of methane by thermal plasma for the production of hydrogen and high value-added carbon black

Maxime Gautier 1 Vandad-Julien Rohani 1 Laurent Fulcheri 1
1 PERSEE - Centre Procédés, Énergies Renouvelables, Systèmes Énergétiques
Abstract : In the prospect of a large scale deployment of Renewable Energy for electricity production, plasmas will definitively be a major option to get tuneable, high temperature enthalpy sources without direct CO2 emissions. This paper focuses on the direct decomposition of methane for the simultaneous synthesis of hydrogen and high value-added carbon black. After a review of gas phase carbon particle nucleation and growth physico-chemical phenomena, a new original model for the plasma decomposition of methane is presented. The model solves a reactive turbulent flow in a 3D geometry. The nucleation is based on a detailed reaction mechanism and the particle growth is handled by a sectional method. This model opens the way towards a better understanding of carbon particles gas phase nucleation and growth and consequently to a fine control of high value-added carbon black grades.
Keywords : CFD Nucleation Growth Population balance model
Type de document :
Article dans une revue
International Journal of Hydrogen Energy, Elsevier, 2017, 42 (47), pp.28140-28156. 〈10.1016/j.ijhydene.2017.09.021〉
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https://hal-mines-paristech.archives-ouvertes.fr/hal-01629530
Contributeur : Brigitte Hanot <>
Soumis le : lundi 6 novembre 2017 - 15:18:05
Dernière modification le : mardi 27 mars 2018 - 16:06:22

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Maxime Gautier, Vandad-Julien Rohani, Laurent Fulcheri. Direct decarbonization of methane by thermal plasma for the production of hydrogen and high value-added carbon black. International Journal of Hydrogen Energy, Elsevier, 2017, 42 (47), pp.28140-28156. 〈10.1016/j.ijhydene.2017.09.021〉. 〈hal-01629530〉

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